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Thesis Issued 2026-09-09 EN

Mineral Interactions in Natural Systems as Shown by The Physical Chemistry of The Aqueous Phase

Author: Md. Yusuf Chowdhury

Abstract

An investigation on the stability of the mineral complexes in soil under natura.l and enriched chemical H ) was environments as (Na , , Ca , Mg , 4 carried on for a period of about six years (1963—1969) through a lysimeter Study involving treatments with Na , and NH 4 The chemical composition of the aqueous phage was determined and was found to reflect processes of mineral transformation and alteration. The aqueous phase of the mineral environment was obtained by two ways (a) displacement under conditions (lysimetry) and (b) pressure extraction . The stability relationship of the phases of the system K C ..—AI O - Sio 2 - H O, Mgo - A1 0 2 - SIO - H 20, and 2 cao - A1 0 - Sio - Sio 2 parameters of H O were studied employing different ionic the aqueous phases. 2 The zonic parameters for soil samples taken from different parts of the profile showed kaolinite to be the In the lower stable phase of the clay mineral complex . part of the profile and samples from Na treated soil layers, a tendency was shown toward the montmorillonite phase. These samples released greater amounts of silica and cations indicating a more intense process of alteration and transformation. The sodium treatment presumably retarded the transformatibn : Na —montmorillonite kaolinite + H SIO + Na as Na is bnézof the products The water samples from the Lysimeters were in contact with the lower part considerable period of time showed the stability phases montmorillonite.. The ionic that were vertically higher kaolihite than those the of the soil profile for a and the ionic parameters of II lite and parameters occupied positions in the field of stability of expressed soil solutions . X—ray analysis of the clay fraction of the soil samples showed the presence Of kaolinite, montmorillonite , micaceous clays, and quartz. Montmorillonite and micaceous clay were apparently not in equilibrium with the ions the aqueous phases. It was concluded that higher concentration of brought about gome structural dissolution of minerals exchange with octahedral and tetrahedr I constituents the mineral. The process gradually decreased with of Increases o 3 e process o surface and e p w ere interlayer cation exchange became dominant. The chemical composition of the aqueous phage depicted the chemistry of the profile. This wag found Zo be a guide for differentiation of the profile. Another subsidiary aspect of this investigation was the mineral nutrient losses by percolation. Soil treatments with ammonium resulted in highest leaching losses. Ammonium acted as mass ion, as well as a source In general the relative ionic losses were in the of H . order of Na > ca > Mg > > A1 and CX->.SO - > Sio The K treatment exhibited the highest percolation while Na treatment showed the minimum. A grass cropping system reduced leaching losses by reducing percolation and increasing removal